Retrieved by E4-util: 2010/02/01,11:45:31 1 0 0 0 9.424100+4 2.389861+2 1 1 59 09441 1451 1 0.000000+0 1.000000+0 0 0 0 69441 1451 2 1.000000+0 2.000000+7 0 0 10 09441 1451 3 0.000000+0 0.000000+0 0 0 471 969441 1451 4 94-Pu-241 IPPE EVAL-MAY06 NIKOLAEV M.N. 9441 1451 5 RUSFOND MANUAL DIST-DEC06 REV0-MAY06 9441 1451 6 ----RUSFOND MATERIAL 9441 9441 1451 7 -----INCIDENT NEUTRON DATA 9441 1451 8 ------ENDF-6 FORMAT 9441 1451 9 RUSFOND DESCRIPTION 9441 1451 10 (see RUSFOND manual for details) 9441 1451 11 9441 1451 12 March2008 rev1: 9441 1451 13 MF3 MT102 was corrected according manual text 9441 1451 14 in energy range 40-100 keV. 9441 1451 15 9441 1451 16 Evaluated data are compiled by the next manner. 9441 1451 17 1. Resolved and unresolved resonsnce regions - according to 9441 1451 18 ENDF/B-VII. 9441 1451 19 2. Total cross section - according to JENDL-3.3. 9441 1451 20 3. Total inelastic scattering cross section, cross section of 9441 1451 21 discret levels and continuum exitation - according to BROND-2. 9441 1451 22 4. (n,2n) and (n,3n) cross sections - accordind to ENDF/B-VII; 9441 1451 23 contribution of (n,4n) cross section is excluded from (n,3n) 9441 1451 24 cross section. 9441 1451 25 5. (n,4n) cross section is taken from JENDL-3.3, but reduced 9441 1451 26 two times. 9441 1451 27 6. Radiative capture cross section - according to BROND-2. 9441 1451 28 7. Fission cross section according to new evaluation (see RUSFOND 9441 1451 29 Manual) 9441 1451 30 8. (n,p) and (n,alfa) cross sections are taken from EAF-2003. 9441 1451 31 9. Elastic scattering cross section is obtained from balance. 9441 1451 32 10.Thermal value of nu-tot is 2.948 in accordance with 2005 9441 1451 33 International Standard Group recommendation; 9441 1451 34 energy dependence of nu-tot - as in JENDL-3.3. 9441 1451 35 11.Number of delayed neutron is adopted the same as in JEFF-3.1. 9441 1451 36 Energy dependence of this number is abcent. 9441 1451 37 8 unuversal group lambda are determined. 9441 1451 38 12.Energy dependence of prompt fission neutrons yield determined 9441 1451 39 as difference between totsl and delayed fission neutron yelds 9441 1451 40 13.Components of energy release due to fission adopted as in 9441 1451 41 ENDF/B-VII . 9441 1451 42 14.Elastic scattering angular distributions are taken from 9441 1451 43 JENDL-3.3. 9441 1451 44 15.Angular distributions of neutrons inelastically scattered with 9441 1451 45 exitation of the first level are taken from BROND-2 9441 1451 46 16.Angular distributions of neutrons inelastically scattered with 9441 1451 47 exitetion of 2-d and 3-rd levels are taken from JENDL-3.3. 9441 1451 48 17.All other angular distributions of secondary neutrons are 9441 1451 49 isotropic in the center of mass system. 9441 1451 50 18.Energy spectra of (n,2n) and (n,3n) neutrons are the same as 9441 1451 51 in ENDF/B-VII . 9441 1451 52 19.Energy spectra of (n,4n) neutrons are the same as in JENDL-3.3.9441 1451 53 20.Fission neutron spectra are taken from JENDL-3.3. 9441 1451 54 21.Energy spectra of neutrons inelastically scattered with 9441 1451 55 exitation of the continuum of levels are taken from BROND-2. 9441 1451 56 22.Parts of delayed neutron groups recommended by JEFF-3.1 are 9441 1451 57 adopted. 9441 1451 58 23.Universal 8 group delayed neutron spectra are the same as in 9441 1451 59 the RUSFOND file for U-235. 9441 1451 60 24.Independent and cumulative fission product yields from 9441 1451 61 ENDF/B-VI are included. 9441 1451 62 9441 1451 63 **************************************************************** 9441 1451 64 COMMENTS TO THE RESONANCE REGION FROM ENDF/B_VIIb2 9441 1451 65 ***************************** JEFF-3.1 *************************9441 1451 66 FEBRUARY 28 2003 9441 1451 67 ---------------------------------------------------------------- 9441 1451 68 Reevaluation of rhe resonance parameters in the energy range up 9441 1451 69 to 20 eV - Colaboration ORNL(USA)-CEN/CAD(FRANCE) 9441 1451 70 H. Derrien and L.C Leal, ORNL 9441 1451 71 A. Courcelle and A. Santamarina, CEN/CAD 9441 1451 72 (submitted to NSE, 2003) 9441 1451 73 9441 1451 74 9441 1451 75 Cross section integrals in the energy range 0.0021 eV to 20.0 eV 9441 1451 76 9441 1451 77 ------------------------------------------------------------- 9441 1451 78 Energy Range Capture b-eV Fission b-eV 9441 1451 79 eV 1993 Present 1993 Present 9441 1451 80 ------------------------------------------------------------- 9441 1451 81 0.0021-0.020 12.25 12.51 2.1% 31.06 31.43 1.2% 9441 1451 82 0.0200-0.030 3.67 3.72 1.4% 10.24 10.36 1.2% 9441 1451 83 0.0300-0.100 15.28 15.59 2.0% 49.02 49.14 0.2% 9441 1451 84 0.1000-0.500 110.58 117.40 6.2% 262.76 263.84 0.4% 9441 1451 85 0.5000-1.000 5.90 6.03 2.2% 17.93 17.89 -0.2% 9441 1451 86 1.0000-3.000 7.30 7.16 -2.0% 54.88 52.89 -3.8% 9441 1451 87 3.0000-20.00 1213. 1234. 1.7% 3039. 3026. -0.4% 9441 1451 88 ------------------------------------------------------------- 9441 1451 89 9441 1451 90 The cross sections at 0.0253 eV are the following: 9441 1451 91 9441 1451 92 Total 1386.5 b 9441 1451 93 Fission 1012.2 b 9441 1451 94 Capture 363.0 b 9441 1451 95 9441 1451 96 very close to the current standard. 9441 1451 97 9441 1451 98 The fit of the experimental data (Young total, Wagemans fission, 9441 1451 99 Weston capture and Weston fission ) were performed by assuming 9441 1451 100 that young total and Wagemans fission were OK with the standard 9441 1451 101 and that Weston original data(from the EXFOR file)needed a renor- 9441 1451 102 zation to agree with the standard. A consistent normalization 9441 1451 103 was obtained by a SAMMY fit leading to a decrease of 4.5% 9441 1451 104 in the original Weston fission and a decrease of 3.0% in the 9441 1451 105 original Weston capture.The differences between the 1988, 1993 9441 1451 106 and the present results are consistent with the experimental 9441 1451 107 errors given by Weston for the measured fission (2-3%) and 9441 1451 108 capture (10-15%). The default of normalization of the Weston 9441 1451 109 fission,due to severe experimental errors in the thermal range, 9441 1451 110 was responsible for the large uncertainty in the capture results. 9441 1451 111 9441 1451 112 9441 1451 113 9441 1451 114 9441 1451 115 ***************************************************************** 9441 1451 116 * * * * * 9441 1451 117 CHANGES FOR REVISION 2 WERE INSERTION OF REVISED RESONANCE REGION9441 1451 118 PARAMETERS BY DERRIEN; RENORMALIZATION OF CAPTURE ABOVE THE 9441 1451 119 RESOLVED RESONANCE REGION TO BE 4.8% LOWER THAN VERSION 5 AND 9441 1451 120 UPWARD FROM 14% DOWN IN ORIGINAL VERSION 6. SCATTERING WAS 9441 1451 121 ADJUSTED TO MAKE UP DIFFERENCE. THE RENORMALIZATION WAS THE 9441 1451 122 SUGGESTION OF DERRIEN AFTER STUDY OF THE NEW MEASUREMENTS BY 9441 1451 123 WAGEMANS ET AL., REF 1. 9441 1451 124 * * * * * 9441 1451 125 PU-241 WAS REVISED FOR VERSION VI BY L.W.WESTON. THE 9441 1451 126 CHANGES WERE THE ADOPTION OF THE RECOMMENDED VALUES OF THE 9441 1451 127 STANDARDS COMMITTEE FOR THE THERMAL CONSTANTS; THE ADOPTION 9441 1451 128 OF THE REICH-MOORE RESONANCE PARAMETER EVALUATION OF THE 9441 1451 129 RESOLVED RESONANCE REGION BY H.DERRIEN,REF 2., OF CADARACHE, 9441 1451 130 FRANCE; RENORMALIZATION OF CAPTURE ABOVE 300EV BY 14% DOWNWARD 9441 1451 131 AS RECOMMENDED BY H.DERRIEN. THE TOTALS ABOVE 100 KEV WERE MADE 9441 1451 132 SAME AS PU-239. CAPTURE REVISED DOWNWARD ABOVE 1.5 MEV. 9441 1451 133 COVARIANCES WERE STRIPED OFF BECAUSE THEY WERE DEPENDANT ON 9441 1451 134 U-235 COVARIANCES WHICH ARE NOT COMPLETED. 9441 1451 135 ******************************************************************9441 1451 136 MF=1 MT=452 THERMAL NUBAR OF 2.9453 RECOMMENDED BY STANDARDS 9441 1451 137 COMMITTEE. PROMPT RATIOS TO CF ABOVE .47 MEV FROM 9441 1451 138 FREHAUT,REF.3. NUBAR PROMPT OF CF OF 3.7676. 9441 1451 139 MF=1 MT=455 TABULATION OF NU DELAYED (REF.4) EXCEPT THERMAL. 9441 1451 140 MF=1 MT=456 SEE MT=452 9441 1451 141 MF=2 MT=151 RESOLVED RESONANCE REGION 10-5 TO 300EV,REICH-MOORE 9441 1451 142 $$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$9441 1451 143 REVISED RESONANCE DATA ,JAERI MAY 1993 9441 1451 144 ***************************************************************** 9441 1451 145 Revision of the 241Pu Reich-Moore resonance parameters 9441 1451 146 by comparison with recent fission cross section measurements. 9441 1451 147 9441 1451 148 Herve Derrien 9441 1451 149 Japanese Atomic Energy Research Institute 9441 1451 150 9441 1451 151 I-INTRODUCTION. 9441 1451 152 The resonance parameters of the neutron cross sections 9441 1451 153 of 241Pu were obtained by Derrien and de Saussure(2) in the energy9441 1451 154 range from thermal to 300 eV by a Bayesian fit of selected 9441 1451 155 experimental effective total cross sections, fission and capture 9441 1451 156 cross sections by using the Reich-Moore fitting code SAMMY(5). 9441 1451 157 The results of this work were used in the ENDF/B-VI evaluated data9441 1451 158 file. Some difficulties were encountered in the normalization of 9441 1451 159 the experimental fission cross sections due to the discrepancies 9441 1451 160 in the shape of the available experimental data both in thermal 9441 1451 161 and high energy ranges. The consistency among the experimental 9441 1451 162 data base could not be obtained without large renormalization and 9441 1451 163 background correction parameters in the SAMMY fits. Particularly,9441 1451 164 it was shown that the discrepancy between the fission cross 9441 1451 165 sections in the thermal energy range was due to a deviation from 9441 1451 166 the 1/v shape below about 0.05 eV. 9441 1451 167 New fission cross section measurements were recently 9441 1451 168 performed by Wagemans et al.(1,6) in the energy range from 0.002 9441 1451 169 eV to 20 eV in order to check the shape of the cross section in 9441 1451 170 the thermal energy range. They showed that the shape of the 9441 1451 171 fission cross section was clearly compatible with the 1/v law,in 9441 1451 172 contradiction to all the previous measurements reported in the 9441 1451 173 literature. Consequently, the normalization of all the 9441 1451 174 previous results using the low energy region could be erroneous. 9441 1451 175 Particularly,the discrepancy observed in the average fission 9441 1451 176 cross section over the 0.26 eV resonance could be due to the 9441 1451 177 errors of normalization in the thermal region. Wagemans et al. 9441 1451 178 compared the ENDF/B-VI data to their new results and concluded 9441 1451 179 that the evaluated data files using the evaluation of Derrien and 9441 1451 180 de Saussure should be revised in the energy range up to 300 eV. 9441 1451 181 9441 1451 182 II-COMMENTS ON ENDF/B-VI EVALUATION. 9441 1451 183 9441 1451 184 In the energy range from 0.01 eV to 3 eV the new data of 9441 1451 185 Wagemans et al. are on average 2.2% smaller than ENDF/B-VI. This 9441 1451 186 difference is mainly due a difference of 3% between the 1976 data 9441 1451 187 of Wagemans et al.(7) and the new values of Wagemans et al. The 9441 1451 188 1976 data of Wagemans et al. were used in the evaluation of 9441 1451 189 Derrien and de Saussure in the low energy region. 9441 1451 190 In the intermediate energy range from 3 eV to 12 eV,the 9441 1451 191 average fission of ENDF/B-VI is in excellent agreement with the 9441 1451 192 new data of Wagemans et al. In this energy range,the SAMMY fits of9441 1451 193 Derrien and de Saussure were performed on the fission cross 9441 1451 194 section of Weston and Todd(8),of Blons(9) and of Migneco et al. 9441 1451 195 (10) with an adjustment of the normalization factor and of the 9441 1451 196 background correction parameters of all the experimental data; the9441 1451 197 agreement between the new data of Wagemans et al. and ENDF/B-VI 9441 1451 198 shows that, at least in this energy range, SAMMY performed on the 9441 1451 199 data of Weston and Todd a renormalization equivalent to that 9441 1451 200 recommended by Wagemans et al.(1). 9441 1451 201 In the higher range up to 300 eV,the SAMMY fits relied 9441 1451 202 mainly on the high resolution measurements of Blons and of 9441 1451 203 Migneco et al. for the accurate determination of the resonance 9441 1451 204 parameters. Quite large normalization coefficients and background9441 1451 205 correction parameters were also needed in this energy range to 9441 1451 206 obtain the consistency between the calculated cross sections and 9441 1451 207 the experimental data. However,the result of the fits was in quite9441 1451 208 good agreement with the data of Weston and Todd normalized to the 9441 1451 209 1976 data of Wagemans et al.in the low energy region, which is 9441 1451 210 also equivalent to the normalization to the 1983 data of Wagemans 9441 1451 211 et al.(11). Since the earlier data of Wagemans et al. should 9441 1451 212 decrease by 3% to be consistent with the new data, it is likely 9441 1451 213 that the ENDF/B-VI fission cross section could be too large by 9441 1451 214 about 3% in the energy range above 12 eV. 9441 1451 215 9441 1451 216 III-REVISION OF THE RESONANCE PARAMETERS. 9441 1451 217 9441 1451 218 An accurate up-dating of the 241Pu resonance parameters 9441 1451 219 could be obtained by renormalizing the fission experimental data 9441 1451 220 base according to the new data of Wagemans et al. and by 9441 1451 221 restarting the SAMMY fits of the new experimental data base, 9441 1451 222 including the high resolution transmission data of Harvey and 9441 1451 223 Simpson(12). Due to lack of time a new SAMMY analysis was 9441 1451 224 performed only in the energy range from 0.002 eV to 3 eV. In the 9441 1451 225 energy range above 3 eV the up-dating was performed by applying 9441 1451 226 some small corrections to the resonance parameters. 9441 1451 227 The SAMMY analysis of the new Wagemans et al. data was 9441 1451 228 performed along with the total cross section of Young and 9441 1451 229 Smith(13) in the energy range from 0.002 eV to 3 eV,by starting 9441 1451 230 with the ENDF/B-VI resonance parameters. Only the parameters of 9441 1451 231 the 3+ resonances at -0.122 eV and at 0.265 eV were adjusted in 9441 1451 232 this energy range. The values of the cross sections calculated 9441 1451 233 at 0.0253 eV are compared to the standard data(14) in Table 1. The9441 1451 234 average total,fission and capture cross sections calculated with 9441 1451 235 the new resonance parameters are displayed on Table 2,3 and 4 with9441 1451 236 the corresponding experimental data and the values obtained from 9441 1451 237 ENDF/B-VI. One should point out that an energy shift of 9441 1451 238 dE/E=+0.00384 was applied to the data of Young and Smith in order 9441 1451 239 to achieve a good consistency with the energy scale of the 9441 1451 240 fission data of Wagemans et al. over the resonance at 0.0265 eV. 9441 1451 241 In the energy range above 3 eV the small corrections 9441 1451 242 applied to the resonance parameters result in a decrease of the 9441 1451 243 average fission cross section and in an increase of the average 9441 1451 244 capture cross section,with a variation of the average total cross 9441 1451 245 section smaller than the errors of the experimental data of Harvey9441 1451 246 and Simpson. The average values of the fission and capture cross 9441 1451 247 sections calculated with the new resonance parameters are shown in9441 1451 248 Table 5 and 6 along with the renormalized fission cross section of9441 1451 249 Weston and Todd and the values calculated from ENDF/B-VI. 9441 1451 250 9441 1451 251 IV-CONCLUSION. 9441 1451 252 9441 1451 253 The results of the recent measurement of the 241Pu fission9441 1451 254 cross section in the energy range from 0.002 eV to 4 eV of 9441 1451 255 Wagemans et al. were used in a new evaluation of the resonance 9441 1451 256 parameters. The accuracy of the calculated cross sections was 9441 1451 257 greatly improved in the resonance at 0.265 eV. The cross sections 9441 1451 258 averaged over this resonance should have the same accuracy as 9441 1451 259 the standard values at 0.0253 eV. In the high energy region up 9441 1451 260 to 300 eV the SAMMY analysis of the new experimental data base 9441 1451 261 obtained by the renormalization of the experimental data is 9441 1451 262 recommended in order to improve the corrections to the resonance 9441 1451 263 parameters performed in the present work. 9441 1451 264 9441 1451 265 9441 1451 266 Table 1 9441 1451 267 9441 1451 268 Cross sections at 0.0253 eV 9441 1451 269 9441 1451 270 ------------------------------------------------------------- 9441 1451 271 Present results ENDF/B-VI Standard(14) 9441 1451 272 ------------------------------------------------------------- 9441 1451 273 Fission 1012.50(-0.0%) 1012.68+-6.58 9441 1451 274 Capture 361.52(+0.1%) 361.29+-4.95 9441 1451 275 Scattering 11.36(-7.1%) 12.17+-2.62 9441 1451 276 Total 1385.38(-0.1%) 1386.14+-8.64 9441 1451 277 ------------------------------------------------------------- 9441 1451 278 9441 1451 279 9441 1451 280 Table 2 9441 1451 281 9441 1451 282 The total cross section integral in the energy range from 9441 1451 283 0.0021 eV to 3 eV. 9441 1451 284 9441 1451 285 ------------------------------------------------------------------9441 1451 286 Energy range Present work ENDF/B-VI Young and Smith(13) 9441 1451 287 (eV) (b.eV) (b.eV) (b.eV) 9441 1451 288 ------------------------------------------------------------------9441 1451 289 0.0021-0.020 43.54 43.09(-1.0%) 43.25(-0.7%) 9441 1451 290 0.0200-0.030 14.03 14.02(-0.1%) 14.01(-0.1%) 9441 1451 291 0.0300-0.100 65.09 66.17(+1.7%) 64.99(-0.1%) 9441 1451 292 0.1000-0.500 378.38 385.27(+1.8%) 380.10(+0.4%) 9441 1451 293 0.5000-1.000 29.74 29.41(-1.1%) 31.19(+4.4%) 9441 1451 294 1.0000-3.000 83.36 83.92(+0.7%) 82.50(-1.0%) 9441 1451 295 ------------------------------------------------------------------9441 1451 296 0.0021-3.000 614.14 621.88(+1.3%) 616.04(+0.3%) 9441 1451 297 ------------------------------------------------------------------9441 1451 298 9441 1451 299 9441 1451 300 Table 3 9441 1451 301 9441 1451 302 The fission cross section integral in the energy range 9441 1451 303 from 0.0021 eV to 3 eV. 9441 1451 304 9441 1451 305 ------------------------------------------------------------------9441 1451 306 Energy range This work ENDF/B-VI Wagemans et al. Weston and Todd9441 1451 307 (eV) (b.eV) (b.eV) (b.eV)(1) (b.eV)(8) 9441 1451 308 ------------------------------------------------------------------9441 1451 309 0.0021-0.020 31.06 30.61(-1.5%) 31.09(+0.1%) 9441 1451 310 0.0200-0.030 10.24 10.22(-0.2%) 10.24( 0.0%) 9441 1451 311 0.0300-0.100 49.02 50.02(+2.0%) 48.70(-0.6%) 9441 1451 312 0.1000-0.500 262.76 270.84(+3.1%) 264.58(+0.7%) 262.53(-0.1%) 9441 1451 313 0.5000-1.000 17.93 17.64(-1.6%) 17.60(-1.8%) 17.67(-1.4%) 9441 1451 314 1.0000-3.000 54.88 55.62(+1.3%) 54.40(-0.9%) 55.06(+0.3%) 9441 1451 315 ------------------------------------------------------------------9441 1451 316 0.0021-3.000 425.89 434.95(+2.1%) 426.61(+0.2%) 9441 1451 317 ------------------------------------------------------------------9441 1451 318 0.1000-3.000 335.57 344.10(+2.5%) 336.58(+0.3%) 335.26(-0.1%) 9441 1451 319 ------------------------------------------------------------------9441 1451 320 Weston and Todd experimental data were normalized to Wagemans et 9441 1451 321 al.(1) in the energy range from 0.1 eV to 12 eV (original EXFOR 9441 1451 322 data multiplied by 0.952). 9441 1451 323 9441 1451 324 9441 1451 325 Table 4 9441 1451 326 9441 1451 327 The capture cross section integral in the energy range from 9441 1451 328 from 0.0021 eV to3 eV. 9441 1451 329 9441 1451 330 -------------------------------------------------------------- 9441 1451 331 Energy range Present work ENDF/B-VI Weston and Todd(8) 9441 1451 332 (eV) (b.eV) (b.eV) (b.eV) 9441 1451 333 -------------------------------------------------------------- 9441 1451 334 0.0021-0.020 12.25 12.28(+0.2%) 9441 1451 335 0.0200-0.030 3.67 3.68(+0.3%) 9441 1451 336 0.0300-0.100 15.28 15.39(+0.7%) 15.27(-0.1%) 9441 1451 337 0.1000-0.500 110.58 109.47(-1.0%) 110.49(-0.1%) 9441 1451 338 0.5000-1.000 5.90 5.87(-0.5%) 6.51 9441 1451 339 1.0000-3.000 7.30 7.14(-2.2%) 8.96 9441 1451 340 -------------------------------------------------------------- 9441 1451 341 0.0021-3.000 154.98 153.83(-0.7%) 9441 1451 342 -------------------------------------------------------------- 9441 1451 343 0.0300-3.000 139.06 137.87(-0.9%) 141.29(+1.6%) 9441 1451 344 -------------------------------------------------------------- 9441 1451 345 Weston and Todd experimental data were normalized to the cal- 9441 1451 346 culated average capture cross section over the resonance at 9441 1451 347 0.264 eV (original EXFOR data multiplied by 0.914); in the 9441 1451 348 energy range from 0.5 eV to 3 eV the experimental data are not 9441 1451 349 accurate due to large corrections for the impurities. 9441 1451 350 9441 1451 351 9441 1451 352 Table 5 9441 1451 353 9441 1451 354 The fission cross section integral in the energy range from 9441 1451 355 3 eV to 300 eV. 9441 1451 356 9441 1451 357 ------------------------------------------------------------------9441 1451 358 Energy range Present work ENDF/B-VI Weston and Todd(8) 9441 1451 359 (eV) (b.eV) (b.eV) (b.eV) 9441 1451 360 ------------------------------------------------------------------9441 1451 361 3- 20 3038.63 3066.37(+0.9%) 3036.23(-0.1%) 9441 1451 362 20- 50 1683.69 1739.68(+3.3%) 1705.50(+1.3%) 9441 1451 363 50-100 1971.15 2030.10(+3.0%) 1931.50(-2.0%) 9441 1451 364 100-200 2554.85 2628.39(+2.9%) 2531.00(-0.9%) 9441 1451 365 200-300 2741.23 2820.75(+2.9%) 2747.00(+0.2%) 9441 1451 366 ------------------------------------------------------------------9441 1451 367 3-300 11989.55 12285.29(+2.5%) 11951.23(-0.3%) 9441 1451 368 ------------------------------------------------------------------9441 1451 369 Weston and Todd experimental data were normalized to Wagemans et 9441 1451 370 al.(1) in the energy range from 0.1 eV to 12 eV (original EXFOR 9441 1451 371 data multiplied by 0.952). 9441 1451 372 9441 1451 373 9441 1451 374 Table 6 9441 1451 375 9441 1451 376 The capture cross section integral in the energy range from 9441 1451 377 3 eV to 300 eV. 9441 1451 378 9441 1451 379 ------------------------------------------------------------------9441 1451 380 Energy range Present work ENDF/B-VI Weston and Todd(8) 9441 1451 381 (eV) (b.eV) (b.eV) (b.eV) 9441 1451 382 ------------------------------------------------------------------9441 1451 383 3- 20 1213.07 1138.52(-6.5%) 1192.90(-1.7%) 9441 1451 384 20- 50 330.34 307.48(-7.5%) 338.09(+2.3%) 9441 1451 385 50-100 605.40 585.88(-3.2%) 594.83(-1.8%) 9441 1451 386 100-200 609.83 581.77(-4.8%) 652.68(+7.0%) 9441 1451 387 200-300 684.97 661.12(-3.6%) 700.53(+2.3%) 9441 1451 388 ------------------------------------------------------------------9441 1451 389 3-300 3443.36 3274.77(-5.1%) 3479.04(+1.0%) 9441 1451 390 ------------------------------------------------------------------9441 1451 391 Weston and Todd experimental data normalized to the calculated 9441 1451 392 average capture cross section over the resonance at 0.265 eV 9441 1451 393 (original EXFOR data multiplied by 0.914). 9441 1451 394 9441 1451 395 $$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$9441 1451 396 9441 1451 397 UNRESOLVED RESONANCE PARAMETERS START AT 300EV. 9441 1451 398 SAME AS VERSION V EXCEPT CAPTURE DOWN BY 4.8% AS 9441 1451 399 PER THE RECOMMENDATION OF H. DERRIEN AFTER THE STUDY9441 1451 400 OF THE WAGEMANS ET AL. DATA, REF 1. REVISION 1 HAD 9441 1451 401 CAPTURE DOWN BY 14% WHICH WAS DECIDED TO BE AN 9441 1451 402 OVERCORRECTION. FISSION IS UNCHANGED FROM VERSION 5 9441 1451 403 WHICH WAS BASED ON DATA OF SIMPSON, REF. 16, JAMES, 9441 1451 404 REF. 17, MIGNECO, REF. 10, BLONS, REF. 9, WESTON, 9441 1451 405 REF. 8, AND CARLSON, REF. 18. 9441 1451 406 MF=3 MT=1 TOTALS WERE REVISED FROM VERSION 5 TO REFLECT MORE 9441 1451 407 PHYSICAL SHAPE AS COMPARED TO PU239. 9441 1451 408 MF=3 MT=2 ADJUSTED TO BE CONSISTENT WITH TOTAL AND OTHER 9441 1451 409 PARTIAL CROSS SECTIONS. 9441 1451 410 MF=3 MT=18 ABOVE 40.2KEV SAME AS VERSION V AND BASED ON BEHRENS9441 1451 411 ,REF.15, KAPPELAR,REF.19, AND SZABO,REF.20, RATIOS 9441 1451 412 TO U235 WITH USE OF ENDF V EVALUATION OF U235. 9441 1451 413 MF=3 MT=102 RENORMALIZED DOWNWARD BY 4.8% FROM VERSION V. SEE 9441 1451 414 UNRESOLVED REGION ABOVE FOR EXPLAINATION. 9441 1451 415 MF=5 MT=16 REVISED BY R.J. HOWERTON FOR VERSION V. 9441 1451 416 MF=5 MT=17 REVISED BY R.J. HOWERTON FOR VERSION V. 9441 1451 417 MF=5 MT=18 FISSION NEUTRON ENERGY DISTRIBUTION GIVEN 9441 1451 418 AS SIMPLE FISSION SPECTRUM PLUS A 9441 1451 419 MAXWELLIAN (AWRE O-101/64) 9441 1451 420 MF=5 MT=91 REVISED BY R.J. HOWERTON FOR VERSION V. 9441 1451 421 MF=5,MT=455 DELAYED NEUTRON SECONDARY ENERGY DISTRIBUTION 9441 1451 422 SEE REF. 21. 9441 1451 423 MF=12 MT=18 USED DATA OF PEELE AND MAIENSCHEIN, REF 22, FOR 9441 1451 424 235-U THERMAL FISSION. 9441 1451 425 MF=12 MT=102 USED 238-U SPECTRUM ADJUSTED FOR MULTIPLICITY AND 9441 1451 426 ENERGY CONSERVATION. 9441 1451 427 MF=13 MT=3 CALCULATED BY R.J. HOWERTON 9441 1451 428 MF=15 MT=3 CALCULATED BY R.J. HOWERTON 9441 1451 429 MF=15 MT=18 CALCULATED BY R.J. HOWERTON. USED PEELE AND 9441 1451 430 MAIENSCHEIN DATA, REF 22, AND METHOD DESCRIBED 9441 1451 431 IN REF 23. 9441 1451 432 MF=15 MT=102 CALCULATED BY R.J. HOWERTON. 9441 1451 433 MF=33 MT=18,102 REPLACED BY L.WESTON DEC.1982 REF.24. 9441 1451 434 9441 1451 435 REFERENCES. 9441 1451 436 9441 1451 437 1. WAGEMANS,C. ET AL., Proc. Int. Conf. Nuc. Data for Sci. and 9441 1451 438 Tech., May 13-17, 1991, Julich, p. 35(1992). 9441 1451 439 2. DERRIEN,H. and de SAUSSURE,G.,Nuc.Sci.Eng.106,415(1990). 9441 1451 440 3. FREHAUT ET AL., CEA-R-4626, BRC(1974). 9441 1451 441 4. KAISER, R.E., CARPENTER, S.G.,(ANL-WEST) private comm.(1977).9441 1451 442 5. LARSON,N.M. and PEREY,F.G.,ORNL/TM-9719(1985). 9441 1451 443 6. WAGEMANS,C.,SCHILLEBEECKX,P.,DERUYTTER,A. and 9441 1451 444 BARTHELEMY,R.,Proc.Int.Conf.,PHYSOR 90,Marseille,France, 9441 1451 445 Vol.1,III-9(1990). 9441 1451 446 7. WAGEMANS,C. and DERUYTTER,A.,Nucl.Sci.Eng.60,44(1976). 9441 1451 447 8. WESTON,L.W. and TODD,J.H.,Nucl.Sci.Eng.65,454(1978). 9441 1451 448 9. BLONS,J.,Nucl.Sci.Eng.51,130(1973). 9441 1451 449 10. 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TO B.A.MAGURNO NOV.12,1982 9441 1451 473 ---------------------------------------------------------------- 9441 1451 474 9441 1451 475 1 451 571 19441 1451 476 1 452 4 09441 1451 477 1 455 8 09441 1451 478 1 456 5 09441 1451 479 1 458 5 09441 1451 480 2 151 409 09441 1451 481 3 1 74 09441 1451 482 3 2 62 09441 1451 483 3 4 37 09441 1451 484 3 16 17 09441 1451 485 3 17 9 09441 1451 486 3 18 40 09441 1451 487 3 37 5 09441 1451 488 3 51 22 09441 1451 489 3 52 21 09441 1451 490 3 53 19 09441 1451 491 3 54 19 09441 1451 492 3 55 19 09441 1451 493 3 56 19 09441 1451 494 3 57 18 09441 1451 495 3 58 18 09441 1451 496 3 59 18 09441 1451 497 3 60 18 09441 1451 498 3 61 17 09441 1451 499 3 62 16 09441 1451 500 3 63 15 09441 1451 501 3 64 15 09441 1451 502 3 65 14 09441 1451 503 3 66 13 09441 1451 504 3 67 12 09441 1451 505 3 68 12 09441 1451 506 3 69 11 09441 1451 507 3 70 12 09441 1451 508 3 71 11 09441 1451 509 3 72 11 09441 1451 510 3 73 10 09441 1451 511 3 74 10 09441 1451 512 3 75 10 09441 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