CENDL-3.1 1 0 0 0 2.204900+4 4.852700+1 1 0 5 12234 1451 1 0.000000+0 0.000000+0 0 0 0 62234 1451 2 1.000000+0 2.000000+7 1 0 10 32234 1451 3 0.000000+0 0.000000+0 0 0 205 492234 1451 4 22-Ti- 49 CNDC EVAL-JAN08 R.R.XU, T.J.LIU, H.C.WU 2234 1451 5 DIST-DEC09 2234 1451 6 ----CENDL-3 MATERIAL 2234 2234 1451 7 -----INCIDENT NEUTRON DATA 2234 1451 8 ------ENDF-6 FORMAT 2234 1451 9 ******************************************************************2234 1451 10 AUTHORS: Rui-Rui XU, Ting-Jin LIU, Hai-Cheng WU, 2234 1451 11 China Nuclear Data Center. 2234 1451 12 ******************************************************************2234 1451 13 HISTORY 2234 1451 14 2008-01 New calculation and evaluation for CENDL-3.1. 2234 1451 15 ************** G E N E R A L I N F O R M A T I O N *************2234 1451 16 2234 1451 17 The natural Titanium and its stable isotopes were newly evaluated 2234 1451 18 in CENDL3.1. The new evaluation files of Ti-49 were derived by the2234 1451 19 following ways: 2234 1451 20 In the first place, we analyzed the experimental data including 2234 1451 21 total, non-elastic scattering cross sections, elastic scattering 2234 1451 22 angular distribution of natural Ti, and the (n,p),(n,np) 2234 1451 23 cross sections of Ti-49. Based on the present analysis results, a 2234 1451 24 set of parameters of Becchetti-Greenlees optical potential model, 2234 1451 25 which is a general optimized one for both the natural Ti and its 2234 1451 26 stable isotopes below 20MeV, was obtained by the code APMN /1/. 2234 1451 27 Then, the direct contributions of discrete energy levels were 2234 1451 28 calculated by the code DWUCK4 /1/, which is constructed by the 2234 1451 29 distorted wave born approximation theory. Guided by the discussed 2234 1451 30 experimental data, both the pre-equilibium and compound nucleus 2234 1451 31 processes below 20MeV were calculated by the code UNF /1/, where 2234 1451 32 the calculated results of DWUCK4 were taken as one input file . 2234 1451 33 In file 2, we utilized the resonance parameters from JENDL3.3, 2234 1451 34 which offers the resolved resonance parameters for MLBW formula 2234 1451 35 in the energy region from 1.0e-5 eV to 180 keV. In file 3, most 2234 1451 36 of the UNF output were adopted except the data of (n,p) 2234 1451 37 reactions,which were substituted by the resluts by fitting the 2234 1451 38 evaluated experimental values with spline function. 2234 1451 39 In the energy region from resonance boundary 2234 1451 40 to 4MeV, the experimental data of (n,tot) cover many 2234 1451 41 unresolved resonances, which didn't appear in our calculation. 2234 1451 42 Furthermore, More experimental data is available for Ti-nat 2234 1451 43 than other isotopes. Then, all our evaluations of 2234 1451 44 (n,tot) were derived though the following ways: for different 2234 1451 45 nuclei, from their own resonant points to 4MeV, the evaluated 2234 1451 46 (n,tot) cross sections employed the same experimental data of 2234 1451 47 Ti-nat, and in the other smooth region the theoretical data were 2234 1451 48 still taken. The elastic scattering angular distributions in file 2234 1451 49 4 were replaced by the outputs of APMN. In order to obtain the 2234 1451 50 evaluated nuclear data files with normalized ENDF/B-VI format and 2234 1451 51 keep the consistency between the different channels,the code 2234 1451 52 CRECTJ6 /2/ was used to compile the modified outputs of UNF. 2234 1451 53 2234 1451 54 Relevant parameters for calculations were completely contained in 2234 1451 55 Ref. /1/. 2234 1451 56 2234 1451 57 ************* D E T A I L E D E V A L U A T I O N **************2234 1451 58 2234 1451 59 mf=1 General information 2234 1451 60 mt=451 Descriptive data and dictionary 2234 1451 61 2234 1451 62 mf=2 Resonance parameters 2234 1451 63 Adopted the resenance parameters from JENDL3.3. 2234 1451 64 mt=151 Resolved resonance parameters 2234 1451 65 Resolved parameters for mlbw formula were given in the energy 2234 1451 66 region from 1.0e-5 eV to 180 keV. Parameters were taken from 2234 1451 67 Ref./3/, for positive resonances. Parameters for negative 2234 1451 68 resonance were obtained so that the reproduced cross sections 2234 1451 69 for both scattering and capture gave the 2200 m/s values of 2234 1451 70 0.7+-0.3 and 2.2+-0.3 barns, respectively/3/. The scattering 2234 1451 71 radius was assumed to be 4.5 fermi instead of 4.0 fermi in 2234 1451 72 Ref./3/. Calculated 2200 m/sec cross sections and resonance 2234 1451 73 integrals are as follows: 2234 1451 74 2234 1451 75 2200 m/s cross section(b) res. integral(b) 2234 1451 76 elastic 0.69 2234 1451 77 capture 1.83 0.89 2234 1451 78 total 2.52 2234 1451 79 2234 1451 80 mf=3 Neutron cross sections 2234 1451 81 Below 180 keV, no background cross section was given. 2234 1451 82 2234 1451 83 ** A set of general parameters for Becchetti-Greenlees optical 2234 1451 84 model was obtained by using APMN, which can search the 2234 1451 85 optimized parameters of Becchetti-Greenlees and Koning 2234 1451 86 optical models rapidly and efficiently by means of the 2234 1451 87 improved fastest falling method. And the total, non-elastic 2234 1451 88 scattering cross sections and elastic angular distribution of 2234 1451 89 Ti-nat were utilized as the criterion in the whole optimizing 2234 1451 90 process. 2234 1451 91 The B-G parameters used in our calculations were: 2234 1451 92 2234 1451 93 V = 49.127-0.486En-0.011En^2-24.0(N-Z)/A, 2234 1451 94 Ws = max{0.0,15.446-0.192En-12.0(N-Z)/A}, 2234 1451 95 Wv = max{0.0, -1.838+0.220En-0.009(N-Z)/A}, 2234 1451 96 Uso= 6.2, 2234 1451 97 Rr = 1.256, Rs = 1.350, Rv = 1.445, Rso= 1.1770, 2234 1451 98 Ar = 0.742, As = 0.323, Av = 0.579, Aso= 0.7500; 2234 1451 99 2234 1451 100 ** The direct contributions of inelastic channel were 2234 1451 101 calculated by DWUCK4,which can perform the zero-range DWBA 2234 1451 102 calculation. For Ti-49 the following discrete levels were 2234 1451 103 taken into account thoughout the inelastic calculations, while2234 1451 104 only the levels marked with '&' were calculated in DWUCK4, and2234 1451 105 the direct contributions of the others were believed to be 2234 1451 106 neglected.The level scheme was taken from Ref./4/. 2234 1451 107 The considered dicrete levels in our calculation: 2234 1451 108 2234 1451 109 no. energy(MeV) spin-parity (direct process) 2234 1451 110 g.s. 0.0 7/2 - 2234 1451 111 1 1.3818 3/2 - & 2234 1451 112 2 1.5421 11/2 - & 2234 1451 113 3 1.586 3/2 - & 2234 1451 114 4 1.6100 9/2 - 2234 1451 115 5 1.6229 5/2 - 2234 1451 116 6 1.7235 1/2 - & 2234 1451 117 2234 1451 118 Levels above 1.7235 MeV were assumed to be overlapping. 2234 1451 119 2234 1451 120 ** The pre-equilibium and compound nucleus processes were 2234 1451 121 calculated by the latest version of UNF, which contains the 2234 1451 122 spherical optical model, the unified Hauser-Feshbach and 2234 1451 123 exciton model. Most data of the file 3 in the new evaluation 2234 1451 124 of Ti-49 adopted the calculation results of UNF except 2234 1451 125 (n,tot),(n,el),(n,non),(n,p),(n,np). More detailed 2234 1451 126 descriptions of this file were listed in the individual 2234 1451 127 channels, respectively. 2234 1451 128 2234 1451 129 mt=1 Total (n,tot) 2234 1451 130 Below 180 keV, created from the resonance parameters; 2234 1451 131 From 180 keV to 4MeV, the recommended experimental data of 2234 1451 132 Ti-nat were adopted instead of the theoretical results. The 2234 1451 133 experimental data were from Ref./5~7/. 2234 1451 134 From 4MeV to 20 MeV, the theoretical data of UNF were 2234 1451 135 adopted. 2234 1451 136 2234 1451 137 mt=2 Elastic scattering (n,el) 2234 1451 138 Constructed by subtracting the sum of the partial cross 2234 1451 139 sections from the total cross section in CRECTJ6. 2234 1451 140 2234 1451 141 mt=3 Non-elastic scattering (n,non) 2234 1451 142 Constructed by summing up the partial cross sections in 2234 1451 143 CRECTJ6. 2234 1451 144 2234 1451 145 mt=4, 51-56, 91 Inelastic scattering 2234 1451 146 Adopted the results of UNF with the direct contributions from 2234 1451 147 DWUCK4. 2234 1451 148 2234 1451 149 mt=16 (n,2n) 2234 1451 150 The calculation of UNF were taken. 2234 1451 151 2234 1451 152 mt=22 (n,na) 2234 1451 153 Calculated cross sections of UNF were utilized in these two 2234 1451 154 channels. 2234 1451 155 2234 1451 156 mt=28 (n,np) 2234 1451 157 The calculation of UNF were taken. 2234 1451 158 2234 1451 159 mt=102 Capture (n,gamma) 2234 1451 160 Below 180 keV, created from the resonance parameters. 2234 1451 161 Above 180 keV, adpoted the calculated results of UNF. 2234 1451 162 2234 1451 163 mt=103 (n,p) 2234 1451 164 Adopted the results by fitting the experimental values, which 2234 1451 165 are mainly fromn the Ref./8,9/ 2234 1451 166 2234 1451 167 mt=104,105,107,111 (n,d), (n,t), (n,a), (n,2p) 2234 1451 168 The calculated results of UNF were taken for the four 2234 1451 169 reactions. 2234 1451 170 2234 1451 171 mf=4 Angular distributions of secondary neutrons 2234 1451 172 mt=2,51-56 2234 1451 173 The calculated angular distributions of UNF were utilized 2234 1451 174 directly. 2234 1451 175 2234 1451 176 mf=6 Energy-angle distributions of secondary particles 2234 1451 177 mt=16, 22, 28, 91 2234 1451 178 Calculated results of UNF were adopted. 2234 1451 179 2234 1451 180 mf=12 Photon production multiplicities and transition probability 2234 1451 181 arrays 2234 1451 182 mt=51-56, 102 2234 1451 183 Calculated results of UNF were adopted. 2234 1451 184 2234 1451 185 mf=14 Photon angular distributions 2234 1451 186 mt=51-56, 102 2234 1451 187 Calculated results of UNF were adopted. 2234 1451 188 2234 1451 189 mf=15 Continuous photon energy spectra 2234 1451 190 mt=102 2234 1451 191 Calculated results of UNF were adopted. 2234 1451 192 2234 1451 193 2234 1451 194 References: 2234 1451 195 1) R.R.Xu, et al., Nuclear Science and Engineering, 334-348, 160 2234 1451 196 (2008). 2234 1451 197 2) Tsuneo NAKAGAWA. CRECTJ: a computer program for compilation 2234 1451 198 of evaluated nuclear data. Japan Atomic Energy Research 2234 1451 199 Institute(1999). 2234 1451 200 3) Mughabghab, S.F. et al. : " Neutron Cross Sections ", Vol.1, 2234 1451 201 Part A (1981). 2234 1451 202 4) 8th edition of the Table of Isotopes: 1998 Update. 2234 1451 203 5) E.Barnard,J.DE Villiers,etc. NP/A,229,189,197409. 2234 1451 204 6) R.B.Schwartz,R.A.Schrack,etc. R,NBS-MONO-138,197401. 2234 1451 205 7) D.G.Foster Jr,D.W.Glasgow. PR/C,3,576,197102. 2234 1451 206 8) H.L.Pai. CJP,44,2337,66. 2234 1451 207 9) Y.Ikeda,C.Konno,etc. S,JAERI-M-91-032,281,9103. 2234 1451 208 ************************ C O N T E N T S ************************ 2234 1451 209 1 451 258 12234 1451 210 2 151 54 02234 1451 211 3 1 715 12234 1451 212 3 2 715 12234 1451 213 3 3 94 12234 1451 214 3 4 45 12234 1451 215 3 16 21 12234 1451 216 3 22 8 12234 1451 217 3 28 11 12234 1451 218 3 51 45 12234 1451 219 3 52 44 12234 1451 220 3 53 43 12234 1451 221 3 54 42 12234 1451 222 3 55 42 12234 1451 223 3 56 41 12234 1451 224 3 91 39 12234 1451 225 3 102 54 12234 1451 226 3 103 52 12234 1451 227 3 104 15 12234 1451 228 3 105 10 12234 1451 229 3 106 6 12234 1451 230 3 107 26 12234 1451 231 3 111 8 12234 1451 232 4 2 554 12234 1451 233 4 51 186 12234 1451 234 4 52 181 12234 1451 235 4 53 181 12234 1451 236 4 54 76 12234 1451 237 4 55 76 12234 1451 238 4 56 181 12234 1451 239 6 16 532 12234 1451 240 6 22 326 12234 1451 241 6 28 428 12234 1451 242 6 91 940 12234 1451 243 12 51 3 12234 1451 244 12 52 3 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2.300000+4 3.000000+0 6.519000+2 6.510000+2 9.000000-1 0.000000+02234 2151 11 2.730000+4 4.000000+0 3.737300+2 3.730000+2 7.300000-1 0.000000+02234 2151 12 3.158000+4 3.000000+0 3.535000+1 3.400000+1 1.350000+0 0.000000+02234 2151 13 3.240000+4 4.000000+0 1.330900+3 1.330000+3 9.000000-1 0.000000+02234 2151 14 3.670000+4 3.000000+0 4.602900+2 4.600000+2 2.900000-1 0.000000+02234 2151 15 3.840000+4 4.000000+0 1.511300+3 1.510000+3 1.300000+0 0.000000+02234 2151 16 5.145000+4 3.000000+0 2.303500+2 2.300000+2 3.500000-1 0.000000+02234 2151 17 5.682000+4 4.000000+0 5.247900+2 5.240000+2 7.900000-1 0.000000+02234 2151 18 6.007000+4 3.000000+0 4.506000+2 4.500000+2 6.000000-1 0.000000+02234 2151 19 6.322000+4 3.000000+0 2.306850+2 2.300000+2 6.850000-1 0.000000+02234 2151 20 6.759990+4 3.000000+0 8.007000+2 8.000000+2 7.000000-1 0.000000+02234 2151 21 7.669990+4 4.000000+0 8.914000+2 8.900000+2 1.400000+0 0.000000+02234 2151 22 9.659990+4 3.000000+0 3.000700+3 3.000000+3 7.000000-1 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