CENDL-3.1 1 0 0 0 2.204600+4 4.555800+1 1 0 5 12225 1451 1 0.000000+0 0.000000+0 0 0 0 62225 1451 2 1.000000+0 2.000000+7 1 0 10 32225 1451 3 0.000000+0 0.000000+0 0 0 209 452225 1451 4 22-Ti- 46 CNDC EVAL-JAN08 R.R.XU, T.J.LIU, H.C.WU 2225 1451 5 DIST-DEC09 2225 1451 6 ----CENDL-3 MATERIAL 2225 2225 1451 7 -----INCIDENT NEUTRON DATA 2225 1451 8 ------ENDF-6 FORMAT 2225 1451 9 ******************************************************************2225 1451 10 AUTHORS: Rui-Rui XU, Ting-Jin LIU, Hai-Cheng WU, 2225 1451 11 China Nuclear Data Center. 2225 1451 12 ******************************************************************2225 1451 13 HISTORY 2225 1451 14 2008-01 New calculation and evaluation for CENDL-3.1. 2225 1451 15 ************** G E N E R A L I N F O R M A T I O N *************2225 1451 16 2225 1451 17 The natural Titanium and its stable isotopes were newly evaluated 2225 1451 18 in CENDL3.1. The new evaluation files of Ti-46 were derived by the2225 1451 19 following ways: 2225 1451 20 In the first place, we analyzed the experimental data including 2225 1451 21 total, non-elastic scattering cross sections, elastic scattering 2225 1451 22 angular distribution of natural Ti, and the (n,p),(n,2n) 2225 1451 23 cross sections of Ti-46. Based on the present analysis results, a 2225 1451 24 set of parameters of Becchetti-Greenlees optical potential model, 2225 1451 25 which is a general optimized one for both the natural Ti and its 2225 1451 26 stable isotopes below 20MeV, was obtained by the code APMN/1/. 2225 1451 27 Then, the direct contributions of discrete energy levels were 2225 1451 28 calculated by the code DWUCK4 /1/, which is constructed by the 2225 1451 29 distorted wave born approximation theory. Guided by the discussed 2225 1451 30 experimental data, both the pre-equilibium and compound nucleus 2225 1451 31 processes below 20MeV were calculated by the code UNF /1/, where 2225 1451 32 the calculated results of DWUCK4 were taken as one input file . 2225 1451 33 In file 2, we utilized the resonance parameters from JENDL3.3, 2225 1451 34 which offers the resolved resonance parameters for MLBW formula 2225 1451 35 in the energy region from 1.0e-5 eV to 300 keV. In file 3, most 2225 1451 36 of the UNF output were adopted except the data of (n,p) and (n,2n)2225 1451 37 reactions,which were substituted by the resluts by fitting the 2225 1451 38 evaluated experimental values with spline function. 2225 1451 39 In the energy region from resonance boundary 2225 1451 40 to 4MeV, the experimental data of (n,tot) cover many 2225 1451 41 unresolved resonances, which didn't appear in our calculation. 2225 1451 42 Furthermore, More experimental data is available for Ti-nat 2225 1451 43 than other isotopes. Then, all our evaluations of 2225 1451 44 (n,tot) were derived though the following ways: for different 2225 1451 45 nuclei, from their own resonant points to 4MeV, the evaluated 2225 1451 46 (n,tot) cross sections employed the same experimental data of 2225 1451 47 Ti-nat, and in the other smooth region the theoretical data were 2225 1451 48 still taken. In order to obtain the 2225 1451 49 evaluated nuclear data files with normalized ENDF/B-VI format and 2225 1451 50 keep the consistency between the different channels,the code 2225 1451 51 CRECTJ6 /2/ was used to compile the modified outputs of UNF. 2225 1451 52 2225 1451 53 Relevant parameters for calculations were completely contained in 2225 1451 54 Ref. /1/. 2225 1451 55 2225 1451 56 ************* D E T A I L E D E V A L U A T I O N **************2225 1451 57 2225 1451 58 mf=1 General information 2225 1451 59 mt=451 Descriptive data and dictionary 2225 1451 60 2225 1451 61 mf=2 Resonance parameters 2225 1451 62 Adopted the resenance parameters from JENDL3.3. 2225 1451 63 mt=151 Resolved resonance parameters 2225 1451 64 Resolved parameters for MLBW formula were given in the energy 2225 1451 65 region from 1.0e-5 eV to 300 keV. Parameters were taken from 2225 1451 66 Ref./3/, for positive resonances. Parameters for negative 2225 1451 67 resonance were obtained so that the reproduced cross sections 2225 1451 68 for both scattering and capture gave the 2200 m/s values of 2225 1451 69 2.78+-0.24 and 0.59+-0.18 barn, respectively/3/. The scatter-2225 1451 70 ing radius was assumed to be 4.5 fermi instead of 3.5 fermi in2225 1451 71 Ref./3/. Calculated 2200 m/sec cross sections and resonance 2225 1451 72 integrals are as follows: 2225 1451 73 2225 1451 74 2200 m/s cross section(b) res. integral(b) 2225 1451 75 elastic 3.68 2225 1451 76 capture 0.576 0.34 2225 1451 77 total 4.26 2225 1451 78 2225 1451 79 mf=3 Neutron cross sections 2225 1451 80 Below 300 keV, no background cross section was given. 2225 1451 81 2225 1451 82 ** A set of general parameters for Becchetti-Greenlees optical 2225 1451 83 model was obtained by using APMN, which can search the 2225 1451 84 optimized parameters of Becchetti-Greenlees and Koning 2225 1451 85 optical models rapidly and efficiently by means of the 2225 1451 86 improved fastest falling method. And the total, non-elastic 2225 1451 87 scattering cross sections and elastic angular distribution of 2225 1451 88 Ti-nat were utilized as the criterion in the whole optimizing 2225 1451 89 process. 2225 1451 90 The B-G parameters used in our calculations were: 2225 1451 91 2225 1451 92 V = 49.127-0.486En-0.011En^2-24.0(N-Z)/A, 2225 1451 93 Ws = max{0.0,15.446-0.192En-12.0(N-Z)/A}, 2225 1451 94 Wv = max{0.0, -1.838+0.220En-0.009(N-Z)/A}, 2225 1451 95 Uso= 6.2, 2225 1451 96 Rr = 1.256, Rs = 1.350, Rv = 1.445, Rso= 1.1770, 2225 1451 97 Ar = 0.742, As = 0.323, Av = 0.579, Aso= 0.7500; 2225 1451 98 2225 1451 99 ** The direct contributions of inelastic channel were 2225 1451 100 calculated by DWUCK4,which can perform the zero-range DWBA 2225 1451 101 calculation. For Ti-46 the following discrete levels were 2225 1451 102 taken into account thoughout the inelastic calculations, while2225 1451 103 only the levels marked with '&' were calculated in DWUCK4, and2225 1451 104 the direct contributions of the others were believed to be 2225 1451 105 neglected.The level scheme was taken from Ref./4/. 2225 1451 106 The considered dicrete levels in our calculation: 2225 1451 107 2225 1451 108 no. energy(MeV) spin-parity (direct process) 2225 1451 109 g.s. 0.0 0+ 2225 1451 110 1 0.8893 2+ & 2225 1451 111 2 2.0098 4+ & 2225 1451 112 3 2.6112 0+ 2225 1451 113 4 2.962 2+ & 2225 1451 114 5 3.0585 3- & 2225 1451 115 2225 1451 116 Levels above 3.0585 MeV were assumed to be overlapping. 2225 1451 117 2225 1451 118 ** The pre-equilibium and compound nucleus processes were 2225 1451 119 calculated by the latest version of UNF, which contains the 2225 1451 120 spherical optical model, the unified Hauser-Feshbach and 2225 1451 121 exciton model. Most data of the file 3 in the new evaluation 2225 1451 122 of Ti-46 adopted the calculation results of UNF except 2225 1451 123 (n,tot),(n,el),(n,non),(n,p),(n,2n). More detailed 2225 1451 124 descriptions of this file were listed in the individual 2225 1451 125 channels, respectively. 2225 1451 126 2225 1451 127 mt=1 Total (n,tot) 2225 1451 128 Below 300 keV, created from the resonance parameters; 2225 1451 129 From 300 keV to 4MeV, the recommended experimental data of 2225 1451 130 Ti-nat were adopted instead of the theoretical results. The 2225 1451 131 experimental data were from Ref./5~7/. 2225 1451 132 From 4MeV to 20 MeV, the theoretical data of UNF were 2225 1451 133 adopted. 2225 1451 134 2225 1451 135 mt=2 Elastic scattering (n,el) 2225 1451 136 Constructed by subtracting the sum of the partial cross 2225 1451 137 sections from the total cross section in CRECTJ6. 2225 1451 138 2225 1451 139 mt=3 Non-elastic scattering (n,non) 2225 1451 140 Constructed by summing up the partial cross sections in 2225 1451 141 CRECTJ6. 2225 1451 142 2225 1451 143 mt=4, 51-55, 91 Inelastic scattering 2225 1451 144 Adopted the results of UNF with the direct contributions from 2225 1451 145 DWUCK4. 2225 1451 146 2225 1451 147 mt=16 (n,2n) 2225 1451 148 Adopted the results by fitting the experimental values, which 2225 1451 149 mainly based on the Ref./8~12/. 2225 1451 150 2225 1451 151 mt=22, 28, (n,na),(n,np) 2225 1451 152 Calculated cross sections of UNF were utilized in these two 2225 1451 153 channels. 2225 1451 154 2225 1451 155 mt=102 Capture (n,gamma) 2225 1451 156 Below 300 keV, created from the resonance parameters. 2225 1451 157 Above 300 keV, adpoted the calculated results of UNF. 2225 1451 158 2225 1451 159 mt=103 (n,p) 2225 1451 160 Adopted the results by fitting the experimental values, which 2225 1451 161 were mainly fromn the Ref./13~17/ 2225 1451 162 2225 1451 163 mt=104,105,107,111 (n,d), (n,t), (n,a), (n,2p) 2225 1451 164 The calculated results of UNF were taken for the four 2225 1451 165 reactions. 2225 1451 166 2225 1451 167 mf=4 Angular distributions of secondary neutrons 2225 1451 168 mt=2,51-55 2225 1451 169 The calculated angular distributions of UNF were utilized 2225 1451 170 directly. 2225 1451 171 2225 1451 172 mf=6 Energy-angle distributions of secondary particles 2225 1451 173 mt=16, 22, 28, 91 2225 1451 174 Calculated results of UNF were adopted. 2225 1451 175 2225 1451 176 mf=12 Photon production multiplicities and transition probability 2225 1451 177 arrays 2225 1451 178 mt=51-55, 102 2225 1451 179 Calculated results of UNF were adopted. 2225 1451 180 2225 1451 181 mf=14 Photon angular distributions 2225 1451 182 mt=51-55, 102 2225 1451 183 Calculated results of UNF were adopted. 2225 1451 184 2225 1451 185 mf=15 Continuous photon energy spectra 2225 1451 186 mt=102 2225 1451 187 Calculated results of UNF were adopted. 2225 1451 188 2225 1451 189 2225 1451 190 References: 2225 1451 191 1) R.R.Xu, et al., Nuclear Science and Engineering, 334-348, 160 2225 1451 192 (2008). 2225 1451 193 2) Tsuneo NAKAGAWA. CRECTJ: a computer program for compilation 2225 1451 194 of evaluated nuclear data. Japan Atomic Energy Research 2225 1451 195 Institute(1999). 2225 1451 196 3) Mughabghab, S.F. et al. : " Neutron Cross Sections ", Vol.1, 2225 1451 197 Part A (1981). 2225 1451 198 4) 8th edition of the Table of Isotopes: 1998 Update. 2225 1451 199 5) E.Barnard,J.DE Villiers,etc. NP/A,229,189,197409. 2225 1451 200 6) R.B.Schwartz,R.A.Schrack,etc. R,NBS-MONO-138,197401. 2225 1451 201 7) D.G.Foster Jr,D.W.Glasgow. PR/C,3,576,197102. 2225 1451 202 8) H.L.Pai, J,CJP,44,2337,66. 2225 1451 203 9) R.J.Prestwood, J,PR,121,1438,6103. 2225 1451 204 10) A.Paulsen, J,AKE,26,34,7508. 2225 1451 205 11) Y.Ikeda, R,JAERI-1312,88. 2225 1451 206 12) J.Csikai, C,82ANTWER,,414,8209. 2225 1451 207 13) D.L.Smith,J.W.Meadows,NSE, 58,314,197511. 2225 1451 208 14) S.K.Ghorai,J.R.Cooper,etc, JNE,25,319,197108. 2225 1451 209 15) LU Hanlin, WANG Dahai,etc, CST,9,(2),113,7505. 2225 1451 210 16) H.L.Pai, CJP,44,2337,66. 2225 1451 211 17) Y.Ikeda,C.Konno,etc, R,JAERI-1312,88. 2225 1451 212 ************************ C O N T E N T S ************************ 2225 1451 213 1 451 258 12225 1451 214 2 151 104 02225 1451 215 3 1 693 12225 1451 216 3 2 693 12225 1451 217 3 3 92 12225 1451 218 3 4 49 12225 1451 219 3 16 21 12225 1451 220 3 22 14 12225 1451 221 3 28 13 12225 1451 222 3 51 49 12225 1451 223 3 52 39 12225 1451 224 3 53 34 12225 1451 225 3 54 32 12225 1451 226 3 55 31 12225 1451 227 3 91 28 12225 1451 228 3 102 54 12225 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5.000000-1 2.052050+3 2.050000+3 2.050000+0 0.000000+02225 2151 6 1.106000+4 5.000000-1 9.048000+1 9.000000+1 4.800000-1 0.000000+02225 2151 7 3.915000+4 5.000000-1 2.506700+2 2.500000+2 6.700000-1 0.000000+02225 2151 8 4.874000+4 5.000000-1 1.626000+3 1.625000+3 1.000000+0 0.000000+02225 2151 9 6.330000+4 5.000000-1 3.502000+3 3.500000+3 2.000000+0 0.000000+02225 2151 10 9.950000+4 5.000000-1 7.070000+1 7.000000+1 7.000000-1 0.000000+02225 2151 11 1.136000+5 5.000000-1 5.350000+1 5.300000+1 5.000000-1 0.000000+02225 2151 12 1.789000+5 5.000000-1 1.302600+3 1.300000+3 2.600000+0 0.000000+02225 2151 13 1.852000+5 5.000000-1 3.501000+3 3.500000+3 1.000000+0 0.000000+02225 2151 14 2.590000+5 5.000000-1 5.013500+2 5.000000+2 1.350000+0 0.000000+02225 2151 15 2.915000+5 5.000000-1 1.001350+3 1.000000+3 1.350000+0 0.000000+02225 2151 16 3.055000+5 5.000000-1 1.001350+3 1.000000+3 1.350000+0 0.000000+02225 2151 17 3.280000+5 5.000000-1 2.001350+3 2.000000+3 1.350000+0 0.000000+02225 2151 18 3.405000+5 5.000000-1 5.013500+2 5.000000+2 1.350000+0 0.000000+02225 2151 19 4.555790+1 0.000000+0 1 0 438 732225 2151 20 3.990000+3 1.500000+0 3.928000-1 2.800000-3 3.900000-1 0.000000+02225 2151 21 1.372000+4 1.500000+0 7.000000-1 3.500000-1 3.500000-1 0.000000+02225 2151 22 2.123000+4 5.000000-1 1.050000+1 1.000000+1 5.000000-1 0.000000+02225 2151 23 2.406000+4 5.000000-1 4.470000-1 6.700000-2 3.800000-1 0.000000+02225 2151 24 2.877000+4 1.500000+0 7.200000-1 6.000000-2 6.600000-1 0.000000+02225 2151 25 3.400000+4 1.500000+0 1.175000+0 7.500000-2 1.100000+0 0.000000+02225 2151 26 3.522000+4 1.500000+0 2.033000+1 2.000000+1 3.300000-1 0.000000+02225 2151 27 4.229000+4 5.000000-1 8.390000+0 8.000000+0 3.900000-1 0.000000+02225 2151 28 4.285000+4 1.500000+0 8.920000+0 8.000000+0 9.200000-1 0.000000+02225 2151 29 4.452000+4 5.000000-1 8.440000+0 8.000000+0 4.400000-1 0.000000+02225 2151 30 4.740000+4 1.500000+0 9.610000+0 9.000000+0 6.100000-1 0.000000+02225 2151 31 4.937000+4 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